Nanofiltration membranes prepared by co-deposition of quercetin-polydopamine for dye desalination performance |
Authors: YAO Zheng, JIN Teng, DONG Liang-liang, ZHANG Chun-fang, BAI Yun-xiang |
Units: Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Materials Engineering, Jiangnan University, Wuxi 214122 |
KeyWords: quercetin;polydopamine;composite nanofiltration membrane;co-deposition;dye desalination; |
ClassificationCode:TQ028.8 |
year,volume(issue):pagination: 2022,42(5):122-128 |
Abstract: |
Composite nanofiltration membranes were prepared by liquid phase co-deposition of quercetin and dopamine method. The effect of the dosge ratio of dopamine to quercetin on the surface properties of membrane active separation layer and the desalinization performance of dye were investigated. The results showed that the co-deposition of quercetin effectively inhibited the formation of polydopamine aggregates and endowed the membrane surface with better uniformity. Meanwhile, the introduction of quercetin made the structure of separation layer much looser, and significantly improved the permeability of the composite nanofiltration membranes, and the dye rejection rate was always above 92%. When the dosge ratio of dopamine to quercetin was 1:1, the pure water permeability of the composite nanofiltration membrane was up to 179.5 L·m-2·h-1·bar-1, the interception of the Congo red was 99.6%, and the selectivity of the Congo red /NaCl reached 58.7. The membranes also showed excellent long-term operation stability. |
Funds: |
国家自然科学基金面上项目,批准号:22075107 |
AuthorIntro: |
姚铮(1997-),女,江苏常州人,硕士生,主要从事膜材料制备及应用研究,E-mail:18362296930@163.com |
Reference: |
[1] Tavangara T, Karimib M, Rezakazemi M, et al. Textile waste, dyes/inorganic salts separation of cerium oxide-loaded loose nanofiltration polyethersulfone membranes[J]. Chemical Engineering Journal, 2020, 385:123787-123800. [2] Liu S B, Wang Z, Ban M, et al. Chelation–assisted in situ self-assembly route to prepare the loose PAN-based nanocomposite membrane for dye desalination[J]. Journal of Membrane Science, 2018, 566:168-180. [3] Zhang Q, Fan L, Yang Z, et al. Loose nanofiltration membrane for dye/salt separation through interfacial polymerization with in-situ generated TiO2 nanoparticles[J]. Applied Surface Science, 2017, 410:494-504. [4] Li Q, Liao Z P, Fang X F, et al. Tannic acid assisted interfacial polymerization based loose thin-film composite NF membrane for dye/salt separation[J]. Desalination, 2020, 479:114343-114352. [5] Saiz-Poseu J, Faraudo J, Figueras A, et al. Switchable Self-Assembly of a Bioinspired Alkyl Catechol at a Solid/Liquid Interface:Competitive Interfacial, Noncovalent, and Solvent Interactions[J]. Chemistry:A European journal, 2012, 18(10):3056-3063. [6] Burzio, Luis A, Waite, et al. Cross-linking in adhesive qumoproteins:studies with model decapeptides[J]. Biochemistry, 2000, 39:11147-11153. [7] Li X L, Zhu L P, Jiang J H, et al. Hydrophilic nanofiltration membranes with self-polymerized and strongly-adhered polydopamine as separating layer[J]. Chinese Journal of Polymer Science, 2012, 30:152–163. [8] Ball V. Physicochemical perspective on "polydopamine" and "poly(catecholamine)" films for their applications in biomaterial coatings[J]. Biointerphases, 2014, 9(3):30801. [9] Xi Z Y, Xu Y Y, Zhu L P, et al. A facile method of surface modification for hydrophobic polymer membranes based on the adhesive behavior of poly(DOPA)and poly(dopamine)[J]. Journal of Membrane Science, 2009, 327:244-253. [10] Wang J, Zhu J Y, Tsehaye M T, et al. High flux electroneutral loose nanofiltration membranes based on rapid deposition of polydopamine/polyethyleneimine[J]. Journal of Materials Chemistry A, 2017, 5:14847-14857. [11] Fei F, Phuong H A L, Blanford C F, et al. Tailoring the performance of organic solvent nanofiltration membranes with biophenol Coatings[J]. ACS Applied Polymer Materials, 2019, 1(3):452-460. [12] Yang H C, Wu M B, Li Y J, et al. Effects of polyethyleneimine molecular weight and proportion on the membrane hydrophilization by codepositing with dopamine[J]. Journal of Applied Polymer Science, 2016, 10:43792-43800. [13] Liu S, Wang Z, Song P. Free radical graft copolymerization strategy to prepare catechin-modified chitosan loose nanofiltration (NF) membrane for dye desalination[J]. ACS Sustainable Chemistry & Engineering, 2018, 6(3):4253-4263. |
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